I am no expert but trying to learn. I think there are drastic changes going on with your water changes. I would let the alk drop gradually to around 7 - 7.2. Are you dosing? Has your alk consumption reduced after the issues have started? Looks like you pretty much did a 100% water change over a period of time. I will stop carbon, as sometimes a high-efficiency carbon will strip off more good stuff than the bad. Running GFO on n off will also be stressing the corals. Just my thoughts.